Characterization of Radio Active Aerosols in Tehran Research Reactor Containment Publisher



Moradi G¹ ; Sadighzadeh A² ; Yarahmadi R³ ; Omidi L¹ ; Farshad AA³ ; Rezaei Fard B²
Source: Nuclear Technology and Radiation Protection Published:2015

Abstract

The objectives of this research were to determine the levels of radioactivity in the Tehran research reactor containment and to investigate the mass-size distribution, composition, and concentration of radio nuclides during operation of the reactor. A cascade impactor sampler was used to determine the size-activity distributions of radioactive aerosols in each of the sampling stations. Levels of α and β activities were determined based on a counting method using a liquid scintillation counter and smear tests. The total average mass fractions of fine particles (particle diameter dp <1 µm) in all of the sampling stations were approximately 26.75 %, with the mean and standard deviation of 52.15 ± 19.75 µg/m3. The total average mass fractions of coarse particles were approximately 73.2%, with the mean and standard deviation of 71.34 ± 24.57 µg/m3. In addition to natural radionuclides, artificial radionuclides, such as 24Na,91Sr,131I,133I,103Ru,82Br, and 140La, may be released into the reactor containment structure. Maximum activity was associated with accumulation-mode particles with diameters less than 400 nm. The results obtained from liquid scintillation counting suggested that the mean specific activity of alpha particles in fine and coarse-modes were 89.7 % and 10.26 %, respectively. The mean specific activity of beta particles in fine and coarse-modes were 81.15 % and 18.51 %, respectively. A large fraction ofthe radionuclides' mass concentration in the Tehran research reactor containment was associated with coarse-mode particles, in addition, a large fraction of the activity in the aerosol particles was associated with accumulation-mode particles. © 2015, Vinca Inst Nuclear Sci. All rights reserved.